Nuclear popcorn: Heavy nucleus changes shapes at different energies

A new paper sheds light on the nature of atomic nuclei.

Everything in the universe, from the largest galaxies down to individual atoms, is governed by four fundamental forces, which together describe how particles interact with each other and make up the world as we know it. These include the electromagnetic force, gravity and the weak and strong nuclear forces.

After a recent study out of the U.S. Department of Energy’s (DOE) Argonne National Laboratory and the University of North Carolina at Chapel Hill, researchers are one step closer to understanding the strong nuclear force, one of the most mysterious of the forces.

“More than 50% of the medical procedures in hospitals today involve nuclear isotopes. And most of these isotopes have been discovered while doing fundamental research like we are doing.” — Robert Janssens, professor, UNC-Chapel Hill

Their work builds on foundational theories of atomic structures that originated with Argonne physicist and Nobel Prize winner Maria Goeppert Mayer in the early 1960s. She helped develop a mathematical model for the structure of nuclei. Her model explained ​why certain numbers of protons and neutrons in the nucleus of an atom cause it to be extremely stable — a phenomenon that had baffled scientists for some time.

The research team previously conducted similar experiments to study the strong nuclear force by examining how the structure of a nucleus can change when it is produced in an excited state through a nuclear reaction. These and other experiments done elsewhere led them to investigate nickel-64, which has 64 neutrons and protons. This nucleus is the heaviest stable nickel nucleus, with 28 protons and 36 neutrons. This nickel isotope has properties that allow its structure to change when it is excited to higher energy states.

For their experiment, the team used the Argonne Tandem Linac Accelerator System, a DOE Office of Science user facility, to accelerate a sample of Ni-64 nuclei toward a target of lead. The lead atoms were able to excite the Ni-64 nuclei through the electromagnetic forces resulting from the repulsion between the protons in lead and the protons in nickel.

The process looks similar to putting a bag of popcorn in the microwave. As the kernels warm up, they begin to pop into all different shapes and sizes. The popcorn that comes out of the microwave is different than what went in and crucially, the kernels changed their shape due to the energy exerted upon them.

After the Ni-64 nuclei were excited, an instrument called GRETINA detected the gamma rays released when the nuclei decayed back to their ground state. Another detector named CHICO2 determined the direction of the particles involved in the interaction. The data obtained by the detectors allowed the team to determine what shape — or shapes — the Ni-64 took as it was excited.

From the analysis of the data, it was concluded that the Ni-64 nuclei excited by interactions with lead also changed their shape. But instead of popping into familiar fluffy shapes, the nickel’s spherical atomic nucleus changed into one of two shapes depending on the amount of energy exerted on it: oblate, like a doorknob, or prolate, like a football. This finding is unusual for heavy nuclei like Ni-64, which consist of many protons and neutrons.

“A model is a picture of reality and it’s only a valid model if it can explain what was known before, and it has some predictive power,” said Robert Janssens, a professor at UNC-Chapel Hill and co-author of the paper. ​“We are studying the nature and behavior of nuclei to continuously improve our current models of the strong nuclear force.”

Ultimately, the researchers hope their findings in Ni-64 and surrounding nuclei can lay the foundations for future practical discoveries in the nuclear science field, such as nuclear energy, astrophysics and medicine. ​“More than 50% of the medical procedures in hospitals today involve nuclear isotopes,” Janssens said. ​“And most of these isotopes have been discovered while doing fundamental research like we are doing.”

A paper based on the research, ​“Multistep Coulomb excitation of ⁶⁴Ni: shape coexistence and nature of low-spin excitations,” was published in October in Physical Review C. This work was part of the Ph.D. thesis project of UNC-Chapel Hill student David Little. A. Daniel Ayangeakaa and Robert Janssens led the UNC efforts, and Michael Carpenter led the Argonne team.

This research was sponsored by the DOE Office of Nuclear Physics, the National Science Foundation.

Argonne National Laboratory seeks solutions to pressing national problems in science and technology. The nation’s first national laboratory, Argonne conducts leading-edge basic and applied scientific research in virtually every scientific discipline. Argonne researchers work closely with researchers from hundreds of companies, universities, and federal, state and municipal agencies to help them solve their specific problems, advance America’s scientific leadership and prepare the nation for a better future. With employees from more than 60 nations, Argonne is managed by UChicago Argonne, LLC for the U.S. Department of Energy’s Office of Science.

The U.S. Department of Energy’s Office of Science is the single largest supporter of basic research in the physical sciences in the United States and is working to address some of the most pressing challenges of our time. For more information, visit https://​ener​gy​.gov/​s​c​ience.